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High-energy, Long-cycle-life Secondary Battery with Electrochemically Pre-doped Silicon Anode.

Abstract：

:Electrochemical pre-doping of a silicon electrode was investigated to create a new class of rechargeable battery with higher energy density. The electrochemical reaction during pre-doping formed a high-quality solid electrolyte interface (SEI) on the surface of silicon particles, which improved the charge and discharge cycle life with a small irreversible capacity. The surface composition of the pre-doped silicon particles was characterized using transmission electron microscopy (TEM), solid state magic-angle-spinning (MAS) nuclear magnetic resonance (NMR) and X-ray diffraction analysis (XRD). Pressurization promoted SEI growth and lithium binding with silicon to form Li15Si4 accompanied by the reductive reaction product of Li2CO3 originated from electrolyte. The Li15Si4 was highly stable when the silicon anode was used in a full cell, thus resulting in a silicon anode with a long cycle life.

journal_name

Sci Rep

journal_title

Scientific reports

authors

Wang Y,Satoh M,Arao M,Matsumoto M,Imai H,Nishihara H

doi

10.1038/s41598-020-59913-4

subject

Has Abstract

pub_date

2020-02-21 00:00:00

pages

3208

issue

1

issn

2045-2322

pii

10.1038/s41598-020-59913-4

journal_volume

10

pub_type

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