Vapor-liquid-solid growth of large-area multilayer hexagonal boron nitride on dielectric substrates.


:Multilayer hexagonal boron nitride (h-BN) is highly desirable as a dielectric substrate for the fabrication of two-dimensional (2D) electronic and optoelectronic devices. However, the controllable synthesis of multilayer h-BN in large areas is still limited in terms of crystallinity, thickness and stacking order. Here, we report a vapor-liquid-solid growth (VLSG) method to achieve uniform multilayer h-BN by using a molten Fe82B18 alloy and N2 as reactants. Liquid Fe82B18 not only supplies boron but also continuously dissociates nitrogen atoms from the N2 vapor to support direct h-BN growth on a sapphire substrate; therefore, the VLSG method delivers high-quality h-BN multilayers with a controllable thickness. Further investigation of the phase evolution of the Fe-B-N system reveals that isothermal segregation dominates the growth of the h-BN. The approach herein demonstrates the feasibility for large-area fabrication of van der Waals 2D materials and heterostructures.


Nat Commun


Nature communications


Shi Z,Wang X,Li Q,Yang P,Lu G,Jiang R,Wang H,Zhang C,Cong C,Liu Z,Wu T,Wang H,Yu Q,Xie X




Has Abstract


2020-02-12 00:00:00












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    authors: Chaguza C,Senghore M,Bojang E,Gladstone RA,Lo SW,Tientcheu PE,Bancroft RE,Worwui A,Foster-Nyarko E,Ceesay F,Okoi C,McGee L,Klugman KP,Breiman RF,Barer MR,Adegbola RA,Antonio M,Bentley SD,Kwambana-Adams BA

    更新日期:2020-07-10 00:00:00

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    更新日期:2013-01-01 00:00:00

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    更新日期:2019-04-04 00:00:00

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    abstract::Conventional rigid electronic systems use a number of metallization layers to route all necessary connections to and from isolated surface mount devices using well-established printed circuit board technology. In contrast, present solutions to prepare stretchable electronic systems are typically confined to a single s...

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    authors: Biswas S,Schoeberl A,Hao Y,Reiprich J,Stauden T,Pezoldt J,Jacobs HO

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    authors: Furtwängler A,Rohrlach AB,Lamnidis TC,Papac L,Neumann GU,Siebke I,Reiter E,Steuri N,Hald J,Denaire A,Schnitzler B,Wahl J,Ramstein M,Schuenemann VJ,Stockhammer PW,Hafner A,Lösch S,Haak W,Schiffels S,Krause J

    更新日期:2020-04-20 00:00:00

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    authors: Wang JX,Irvine MW,Burnell ES,Sapkota K,Thatcher RJ,Li M,Simorowski N,Volianskis A,Collingridge GL,Monaghan DT,Jane DE,Furukawa H

    更新日期:2020-01-22 00:00:00

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    abstract::Broomcorn millet (Panicum miliaceum L.) is the most water-efficient cereal and one of the earliest domesticated plants. Here we report its high-quality, chromosome-scale genome assembly using a combination of short-read sequencing, single-molecule real-time sequencing, Hi-C, and a high-density genetic map. Phylogeneti...

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    authors: Zou C,Li L,Miki D,Li D,Tang Q,Xiao L,Rajput S,Deng P,Peng L,Jia W,Huang R,Zhang M,Sun Y,Hu J,Fu X,Schnable PS,Chang Y,Li F,Zhang H,Feng B,Zhu X,Liu R,Schnable JC,Zhu JK,Zhang H

    更新日期:2019-01-25 00:00:00

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    authors: Fouragnan E,Retzler C,Mullinger K,Philiastides MG

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    authors: Hesketh EL,Saunders K,Fisher C,Potze J,Stanley J,Lomonossoff GP,Ranson NA

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    authors: Damman R,Schütz S,Luo Y,Weingarth M,Sprangers R,Baldus M

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  • Rapid mechanochemical encapsulation of biocatalysts into robust metal-organic frameworks.

    abstract::Metal-organic frameworks (MOFs) have recently garnered consideration as an attractive solid substrate because the highly tunable MOF framework can not only serve as an inert host but also enhance the selectivity, stability, and/or activity of the enzymes. Herein, we demonstrate the advantages of using a mechanochemica...

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    authors: Theodorou P,Radzevičiūtė R,Lentendu G,Kahnt B,Husemann M,Bleidorn C,Settele J,Schweiger O,Grosse I,Wubet T,Murray TE,Paxton RJ

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    authors: Cai Y,Roslund J,Ferrini G,Arzani F,Xu X,Fabre C,Treps N

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    authors: Montaldo NP,Bordin DL,Brambilla A,Rösinger M,Fordyce Martin SL,Bjørås KØ,Bradamante S,Aas PA,Furrer A,Olsen LC,Kunath N,Otterlei M,Sætrom P,Bjørås M,Samson LD,van Loon B

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