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Towards full-colour tunability of inorganic electrochromic devices using ultracompact fabry-perot nanocavities.

Abstract：

:Intercalation-based inorganic materials that change their colours upon ion insertion/extraction lay an important foundation for existing electrochromic technology. However, using only such inorganic electrochromic materials, it is very difficult to achieve the utmost goal of full-colour tunability for future electrochromic technology mainly due to the absence of structural flexibility. Herein, we demonstrate an ultracompact asymmetric Fabry-Perot (F-P) nanocavity-type electrochromic device formed by using partially reflective metal tungsten as the current collector and reflector layer simultaneously; this approach enables fairly close matching of the reflections at both interfaces of the WO3 thin layer in device form, inducing a strong interference. Such an interference-enhanced device that is optically manipulated at the nanoscale displays various structural colours before coloration and, further, can change to other colours including blue, red, and yellow by changing the optical indexes (n, k) of the tungsten oxide layer through ion insertion.

journal_name

Nat Commun

journal_title

Nature communications

authors

Wang Z,Wang X,Cong S,Chen J,Sun H,Chen Z,Song G,Geng F,Chen Q,Zhao Z

doi

10.1038/s41467-019-14194-y

subject

Has Abstract

pub_date

2020-01-16 00:00:00

pages

302

issue

1

issn

2041-1723

pii

10.1038/s41467-019-14194-y

journal_volume

11

pub_type

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