Extreme-ultraviolet high-harmonic generation in liquids.

Abstract:

:High-harmonic generation (HHG) in gases has been the main enabling technology of attosecond science since its discovery. Recently, HHG from solids has been demonstrated, opening a lively area of research. In contrast, harmonic generation from liquids has so far remained restricted to low harmonics in the visible regime. Here, we report the observation and detailed characterization of extreme ultraviolet HHG from liquid water and several alcohols extending beyond 20 eV. This advance was enabled by the implementation of the recent liquid flat-microjet technology, which we show to facilitate the spatial separation of HHG from the bulk liquid and the surrounding gas phase. We observe striking differences between the HHG spectra of water and several alcohols. A comparison with a strongly-driven few-band model establishes the sensitivity of HHG to the electronic structure of liquids. Our results suggest liquid-phase high-harmonic spectroscopy as a new method for studying the electronic structure and ultrafast scattering processes in liquids.

journal_name

Nat Commun

journal_title

Nature communications

authors

Luu TT,Yin Z,Jain A,Gaumnitz T,Pertot Y,Ma J,Wörner HJ

doi

10.1038/s41467-018-06040-4

subject

Has Abstract

pub_date

2018-09-13 00:00:00

pages

3723

issue

1

issn

2041-1723

pii

10.1038/s41467-018-06040-4

journal_volume

9

pub_type

杂志文章
  • Efficient solar-driven electrocatalytic CO2 reduction in a redox-medium-assisted system.

    abstract::Solar-driven electrochemical carbon dioxide (CO2) reduction is capable of producing value-added chemicals and represents a potential route to alleviate carbon footprint in the global environment. However, the ever-changing sunlight illumination presents a substantial impediment of maintaining high electrocatalytic eff...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-07380-x

    authors: Wang Y,Liu J,Wang Y,Wang Y,Zheng G

    更新日期:2018-11-27 00:00:00

  • Female song is widespread and ancestral in songbirds.

    abstract::Bird song has historically been considered an almost exclusively male trait, an observation fundamental to the formulation of Darwin's theory of sexual selection. Like other male ornaments, song is used by male songbirds to attract females and compete with rivals. Thus, bird song has become a textbook example of the p...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms4379

    authors: Odom KJ,Hall ML,Riebel K,Omland KE,Langmore NE

    更新日期:2014-03-04 00:00:00

  • Deformation-induced trace element redistribution in zircon revealed using atom probe tomography.

    abstract::Trace elements diffuse negligible distances through the pristine crystal lattice in minerals: this is a fundamental assumption when using them to decipher geological processes. For example, the reliable use of the mineral zircon (ZrSiO4) as a U-Th-Pb geochronometer and trace element monitor requires minimal radiogenic...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms10490

    authors: Piazolo S,La Fontaine A,Trimby P,Harley S,Yang L,Armstrong R,Cairney JM

    更新日期:2016-02-12 00:00:00

  • Multi-level chirality in liquid crystals formed by achiral molecules.

    abstract::Complex materials often exhibit a hierarchical structure with an intriguing mechanism responsible for the 'propagation' of order from the molecular to the nano- or micro-scale level. In particular, the chirality of biological molecules such as nucleic acids and amino acids is responsible for the helical structure of D...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-019-09862-y

    authors: Salamończyk M,Vaupotič N,Pociecha D,Walker R,Storey JMD,Imrie CT,Wang C,Zhu C,Gorecka E

    更新日期:2019-04-23 00:00:00

  • EGFL7 reduces CNS inflammation in mouse.

    abstract::Extracellular matrix (ECM) proteins secreted by blood-brain barrier (BBB) endothelial cells (ECs) are implicated in cell trafficking. We discovered that the expression of ECM epidermal growth factor-like protein 7 (EGFL7) is increased in the CNS vasculature of patients with multiple sclerosis (MS), and in mice with ex...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-03186-z

    authors: Larochelle C,Uphaus T,Broux B,Gowing E,Paterka M,Michel L,Dudvarski Stankovic N,Bicker F,Lemaître F,Prat A,Schmidt MHH,Zipp F

    更新日期:2018-02-26 00:00:00

  • Amplification of heat extremes by plant CO2 physiological forcing.

    abstract::Plants influence extreme heat events by regulating land-atmosphere water and energy exchanges. The contribution of plants to changes in future heat extremes will depend on the responses of vegetation growth and physiology to the direct and indirect effects of elevated CO2. Here we use a suite of earth system models to...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-03472-w

    authors: Skinner CB,Poulsen CJ,Mankin JS

    更新日期:2018-03-15 00:00:00

  • Human NK cell development requires CD56-mediated motility and formation of the developmental synapse.

    abstract::While distinct stages of natural killer (NK) cell development have been defined, the molecular interactions that shape human NK cell maturation are poorly understood. Here we define intercellular interactions between developing NK cells and stromal cells which, through contact-dependent mechanisms, promote the generat...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms12171

    authors: Mace EM,Gunesch JT,Dixon A,Orange JS

    更新日期:2016-07-20 00:00:00

  • An integrated chromatin accessibility and transcriptome landscape of human pre-implantation embryos.

    abstract::Human pre-implantation embryonic development involves extensive changes in chromatin structure and transcriptional activity. Here, we report on LiCAT-seq, a technique that enables simultaneous profiling of chromatin accessibility and gene expression with ultra-low input of cells, and map the chromatin accessibility an...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-08244-0

    authors: Liu L,Leng L,Liu C,Lu C,Yuan Y,Wu L,Gong F,Zhang S,Wei X,Wang M,Zhao L,Hu L,Wang J,Yang H,Zhu S,Chen F,Lu G,Shang Z,Lin G

    更新日期:2019-01-21 00:00:00

  • Author Correction: Targeting QKI-7 in vivo restores endothelial cell function in diabetes.

    abstract::An amendment to this paper has been published and can be accessed via a link at the top of the paper. ...

    journal_title:Nature communications

    pub_type: 杂志文章,已发布勘误

    doi:10.1038/s41467-020-18712-1

    authors: Yang C,Eleftheriadou M,Kelaini S,Morrison T,González MV,Caines R,Edwards N,Yacoub A,Edgar K,Moez A,Ivetic A,Zampetaki A,Zeng L,Wilkinson FL,Lois N,Stitt AW,Grieve DJ,Margariti A

    更新日期:2020-09-16 00:00:00

  • High-pressure synthesis of a polyethylene/zeolite nano-composite material.

    abstract::Meso/micro-porous solids, such as zeolites, are complex materials used in an impressive range of applications. Here we photo-polymerized ethylene using non-catalytic high-pressure techniques at 0.5-1.5 GPa under ultraviolet (351-364 nm) irradiation on a sub-nanometre scale in the channels of a pure SiO2 zeolite, silic...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms2564

    authors: Santoro M,Gorelli FA,Bini R,Haines J,van der Lee A

    更新日期:2013-01-01 00:00:00

  • SREBP1 drives Keratin-80-dependent cytoskeletal changes and invasive behavior in endocrine-resistant ERα breast cancer.

    abstract::Approximately 30% of ERα breast cancer patients relapse with metastatic disease following adjuvant endocrine therapies. The connection between acquisition of drug resistance and invasive potential is poorly understood. In this study, we demonstrate that the type II keratin topological associating domain undergoes epig...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-019-09676-y

    authors: Perone Y,Farrugia AJ,Rodríguez-Meira A,Győrffy B,Ion C,Uggetti A,Chronopoulos A,Marrazzo P,Faronato M,Shousha S,Davies C,Steel JH,Patel N,Del Rio Hernandez A,Coombes C,Pruneri G,Lim A,Calvo F,Magnani L

    更新日期:2019-05-09 00:00:00

  • Atomically precise edge chlorination of nanographenes and its application in graphene nanoribbons.

    abstract::Chemical functionalization is one of the most powerful and widely used strategies to control the properties of nanomaterials, particularly in the field of graphene. However, the ill-defined structure of the present functionalized graphene inhibits atomically precise structural characterization and structure-correlated...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms3646

    authors: Tan YZ,Yang B,Parvez K,Narita A,Osella S,Beljonne D,Feng X,Müllen K

    更新日期:2013-01-01 00:00:00

  • Fishing for newly synthesized proteins with phosphonate-handles.

    abstract::Bioorthogonal chemistry introduces affinity-labels into biomolecules with minimal disruption to the original system and is widely applicable in a range of contexts. In proteomics, immobilized metal affinity chromatography (IMAC) enables enrichment of phosphopeptides with extreme sensitivity and selectivity. Here, we a...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-020-17010-0

    authors: Kleinpenning F,Steigenberger B,Wu W,Heck AJR

    更新日期:2020-06-26 00:00:00

  • Probing low-energy hyperbolic polaritons in van der Waals crystals with an electron microscope.

    abstract::Van der Waals materials exhibit intriguing structural, electronic, and photonic properties. Electron energy loss spectroscopy within scanning transmission electron microscopy allows for nanoscale mapping of such properties. However, its detection is typically limited to energy losses in the eV range-too large for prob...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-017-00056-y

    authors: Govyadinov AA,Konečná A,Chuvilin A,Vélez S,Dolado I,Nikitin AY,Lopatin S,Casanova F,Hueso LE,Aizpurua J,Hillenbrand R

    更新日期:2017-07-21 00:00:00

  • The telomere binding protein Pot1 maintains haematopoietic stem cell activity with age.

    abstract::Repeated cell divisions and aging impair stem cell function. However, the mechanisms by which this occurs are not fully understood. Here we show that protection of telomeres 1A (Pot1a), a component of the Shelterin complex that protects telomeres, improves haematopoietic stem cell (HSC) activity during aging. Pot1a is...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-017-00935-4

    authors: Hosokawa K,MacArthur BD,Ikushima YM,Toyama H,Masuhiro Y,Hanazawa S,Suda T,Arai F

    更新日期:2017-10-06 00:00:00

  • Quantifying climate sensitivity and climate-driven change in North American amphibian communities.

    abstract::Changing climate will impact species' ranges only when environmental variability directly impacts the demography of local populations. However, measurement of demographic responses to climate change has largely been limited to single species and locations. Here we show that amphibian communities are responsive to clim...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-06157-6

    authors: Miller DAW,Grant EHC,Muths E,Amburgey SM,Adams MJ,Joseph MB,Waddle JH,Johnson PTJ,Ryan ME,Schmidt BR,Calhoun DL,Davis CL,Fisher RN,Green DM,Hossack BR,Rittenhouse TAG,Walls SC,Bailey LL,Cruickshank SS,Fellers GM,G

    更新日期:2018-09-25 00:00:00

  • The Arabidopsis NOT4A E3 ligase promotes PGR3 expression and regulates chloroplast translation.

    abstract::Chloroplast function requires the coordinated action of nuclear- and chloroplast-derived proteins, including several hundred nuclear-encoded pentatricopeptide repeat (PPR) proteins that regulate plastid mRNA metabolism. Despite their large number and importance, regulatory mechanisms controlling PPR expression are poo...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-020-20506-4

    authors: Bailey M,Ivanauskaite A,Grimmer J,Akintewe O,Payne AC,Osborne R,Labandera AM,Etherington RD,Rantala M,Baginsky S,Mulo P,Gibbs DJ

    更新日期:2021-01-11 00:00:00

  • The mTORC1 effectors S6K1 and 4E-BP play different roles in CNS axon regeneration.

    abstract::Using mouse optic nerve (ON) crush as a CNS injury model, we and others have found that activation of the mammalian target of rapamycin complex 1 (mTORC1) in mature retinal ganglion cells by deletion of the negative regulators, phosphatase and tensin homologue (PTEN), and tuberous sclerosis 1 promotes ON regeneration....

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms6416

    authors: Yang L,Miao L,Liang F,Huang H,Teng X,Li S,Nuriddinov J,Selzer ME,Hu Y

    更新日期:2014-11-10 00:00:00

  • Full-field implementation of a perfect eavesdropper on a quantum cryptography system.

    abstract::Quantum key distribution (QKD) allows two remote parties to grow a shared secret key. Its security is founded on the principles of quantum mechanics, but in reality it significantly relies on the physical implementation. Technological imperfections of QKD systems have been previously explored, but no attack on an esta...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms1348

    authors: Gerhardt I,Liu Q,Lamas-Linares A,Skaar J,Kurtsiefer C,Makarov V

    更新日期:2011-06-14 00:00:00

  • Selective photocatalytic conversion of methane into carbon monoxide over zinc-heteropolyacid-titania nanocomposites.

    abstract::Chemical utilization of vast fossil and renewable feedstocks of methane remains one of the most important challenges of modern chemistry. Herein, we report direct and selective methane photocatalytic oxidation at ambient conditions into carbon monoxide, which is an important chemical intermediate and a platform molecu...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-019-08525-2

    authors: Yu X,De Waele V,Löfberg A,Ordomsky V,Khodakov AY

    更新日期:2019-02-11 00:00:00

  • Somatic mutations in clonally expanded cytotoxic T lymphocytes in patients with newly diagnosed rheumatoid arthritis.

    abstract::Somatic mutations contribute to tumorigenesis. Although these mutations occur in all proliferating cells, their accumulation under non-malignant conditions, such as in autoimmune disorders, has not been investigated. Here, we show that patients with newly diagnosed rheumatoid arthritis have expanded CD8+ T-cell clones...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms15869

    authors: Savola P,Kelkka T,Rajala HL,Kuuliala A,Kuuliala K,Eldfors S,Ellonen P,Lagström S,Lepistö M,Hannunen T,Andersson EI,Khajuria RK,Jaatinen T,Koivuniemi R,Repo H,Saarela J,Porkka K,Leirisalo-Repo M,Mustjoki S

    更新日期:2017-06-21 00:00:00

  • 4D Visualization of replication foci in mammalian cells corresponding to individual replicons.

    abstract::Since the pioneering proposal of the replicon model of DNA replication 50 years ago, the predicted replicons have not been identified and quantified at the cellular level. Here, we combine conventional and super-resolution microscopy of replication sites in live and fixed cells with computational image analysis. We co...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms11231

    authors: Chagin VO,Casas-Delucchi CS,Reinhart M,Schermelleh L,Markaki Y,Maiser A,Bolius JJ,Bensimon A,Fillies M,Domaing P,Rozanov YM,Leonhardt H,Cardoso MC

    更新日期:2016-04-07 00:00:00

  • Bio-inspired sensitive and reversible mechanochromisms via strain-dependent cracks and folds.

    abstract::A number of marine organisms use muscle-controlled surface structures to achieve rapid changes in colour and transparency with outstanding reversibility. Inspired by these display tactics, we develop analogous deformation-controlled surface-engineering approaches via strain-dependent cracks and folds to realize the fo...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms11802

    authors: Zeng S,Zhang D,Huang W,Wang Z,Freire SG,Yu X,Smith AT,Huang EY,Nguon H,Sun L

    更新日期:2016-07-08 00:00:00

  • Seasonal energy exchange in sea ice retreat regions contributes to differences in projected Arctic warming.

    abstract::Rapid and, in many cases, unprecedented Arctic climate changes are having far-reaching impacts on natural and human systems. Despite state-of-the-art climate models capturing the rapid nature of Arctic climate change, termed Arctic amplification, they significantly disagree on its magnitude. Using a regional, process-...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-07061-9

    authors: Boeke RC,Taylor PC

    更新日期:2018-11-27 00:00:00

  • MicroRNA-155 influences B-cell function through PU.1 in rheumatoid arthritis.

    abstract::MicroRNA-155 (miR-155) is an important regulator of B cells in mice. B cells have a critical role in the pathogenesis of rheumatoid arthritis (RA). Here we show that miR-155 is highly expressed in peripheral blood B cells from RA patients compared with healthy individuals, particularly in the IgD-CD27- memory B-cell p...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms12970

    authors: Alivernini S,Kurowska-Stolarska M,Tolusso B,Benvenuto R,Elmesmari A,Canestri S,Petricca L,Mangoni A,Fedele AL,Di Mario C,Gigante MR,Gremese E,McInnes IB,Ferraccioli G

    更新日期:2016-09-27 00:00:00

  • Breather soliton dynamics in microresonators.

    abstract::The generation of temporal cavity solitons in microresonators results in coherent low-noise optical frequency combs that are critical for applications in spectroscopy, astronomy, navigation or telecommunications. Breather solitons also form an important part of many different classes of nonlinear wave systems, manifes...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms14569

    authors: Yu M,Jang JK,Okawachi Y,Griffith AG,Luke K,Miller SA,Ji X,Lipson M,Gaeta AL

    更新日期:2017-02-24 00:00:00

  • CHML promotes liver cancer metastasis by facilitating Rab14 recycle.

    abstract::Metastasis-associated recurrence is the major cause of poor prognosis in hepatocellular carcinoma (HCC), however, the underlying mechanisms remain largely elusive. In this study, we report that expression of choroideremia-like (CHML) is increased in HCC, associated with poor survival, early recurrence and more satelli...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-019-10364-0

    authors: Chen TW,Yin FF,Yuan YM,Guan DX,Zhang E,Zhang FK,Jiang H,Ma N,Wang JJ,Ni QZ,Qiu L,Feng J,Zhang XL,Bao Y,Wang K,Cheng SQ,Wang XF,Wang X,Li JJ,Xie D

    更新日期:2019-06-07 00:00:00

  • Crystalline TiO2 protective layer with graded oxygen defects for efficient and stable silicon-based photocathode.

    abstract::The trade-offs between photoelectrode efficiency and stability significantly hinder the practical application of silicon-based photoelectrochemical devices. Here, we report a facile approach to decouple the trade-offs of silicon-based photocathodes by employing crystalline TiO2 with graded oxygen defects as protection...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-05580-z

    authors: Zheng J,Lyu Y,Wang R,Xie C,Zhou H,Jiang SP,Wang S

    更新日期:2018-09-03 00:00:00

  • Hemocyanin facilitates lignocellulose digestion by wood-boring marine crustaceans.

    abstract::Woody (lignocellulosic) plant biomass is an abundant renewable feedstock, rich in polysaccharides that are bound into an insoluble fiber composite with lignin. Marine crustacean woodborers of the genus Limnoria are among the few animals that can survive on a diet of this recalcitrant material without relying on gut re...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-07575-2

    authors: Besser K,Malyon GP,Eborall WS,Paro da Cunha G,Filgueiras JG,Dowle A,Cruz Garcia L,Page SJ,Dupree R,Kern M,Gomez LD,Li Y,Elias L,Sabbadin F,Mohamad SE,Pesante G,Steele-King C,Ribeiro de Azevedo E,Polikarpov I,Dupree

    更新日期:2018-12-03 00:00:00

  • Large bipolaron density at organic semiconductor/electrode interfaces.

    abstract::Bipolaron states, in which two electrons or two holes occupy a single molecule or conjugated polymer segment, are typically considered to be negligible in organic semiconductor devices due to Coulomb repulsion between the two charges. Here we use charge modulation spectroscopy to reveal a bipolaron sheet density >1010...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-017-02459-3

    authors: Dhanker R,Gray CL,Mukhopadhyay S,Nunez S,Cheng CY,Sokolov AN,Giebink NC

    更新日期:2017-12-21 00:00:00