Macroscopic phase separation of superconductivity and ferromagnetism in Sr0.5Ce0.5FBiS2-x Se x revealed by μSR.

Abstract:

:The compound Sr0.5Ce0.5FBiS2 belongs to the intensively studied family of layered BiS2 superconductors. It attracts special attention because superconductivity at T sc  = 2.8 K was found to coexist with local-moment ferromagnetic order with a Curie temperature T C  = 7.5 K. Recently it was reported that upon replacing S by Se T C drops and ferromagnetism becomes of an itinerant nature. At the same time T sc increases and it was argued superconductivity coexists with itinerant ferromagnetism. Here we report a muon spin rotation and relaxation study (μSR) conducted to investigate the coexistence of superconductivity and ferromagnetic order in Sr0.5Ce0.5FBiS2-x Se x with x = 0.5 and 1.0. By inspecting the muon asymmetry function we find that both phases do not coexist on the microscopic scale, but occupy different sample volumes. For x = 0.5 and x = 1.0 we find a ferromagnetic volume fraction of ~8 % and ~30 % at T = 0.25 K, well below T C  = 3.4 K and T C  = 3.3 K, respectively. For x = 1.0 (T sc  = 2.9 K) the superconducting phase occupies most (~64 %) of the remaining sample volume, as shown by transverse field experiments that probe the Gaussian damping due to the vortex lattice. We conclude ferromagnetism and superconductivity are macroscopically phase separated.

journal_name

Sci Rep

journal_title

Scientific reports

authors

Nikitin AM,Grinenko V,Sarkar R,Orain JC,Salis MV,Henke J,Huang YK,Klauss HH,Amato A,Visser A

doi

10.1038/s41598-017-17637-y

subject

Has Abstract

pub_date

2017-12-12 00:00:00

pages

17370

issue

1

issn

2045-2322

pii

10.1038/s41598-017-17637-y

journal_volume

7

pub_type

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