Abstract：
:Kinetic restriction of a thermodynamically favourable equilibrium is a common theme in materials processing. The interfacial instability in systems where rate of material exchange is far greater than the mass transfer through respective bulk phases is of specific interest when tracking the transient interfacial area, a parameter integral to short processing times for productivity streamlining in all manufacturing where interfacial reaction occurs. This is even more pertinent in high-temperature systems for energy and cost savings. Here the quantified physical pathway of interfacial area change due to material exchange in liquid metal-molten oxide systems is presented. In addition the predicted growth regime and emulsification behaviour in relation to interfacial tension as modelled using phase-field methodology is shown. The observed in-situ emulsification behaviour links quantitatively the geometry of perturbations as a validation method for the development of simulating the phenomena. Thus a method is presented to both predict and engineer the formation of micro emulsions to a desired specification.
journal_name
Sci Repjournal_title
Scientific reportsauthors
Spooner S,Rahnama A,Warnett JM,Williams MA,Li Z,Sridhar Sdoi
10.1038/s41598-017-14638-9subject
Has Abstractpub_date
2017-10-30 00:00:00pages
14384issue
1issn
2045-2322pii
10.1038/s41598-017-14638-9journal_volume
7pub_type
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