Missing magnetism in Sr4Ru3O10: Indication for Antisymmetric Exchange Interaction.

Abstract:

:Metamagnetism occuring inside a ferromagnetic phase is peculiar. Therefore, Sr4Ru3O10, a T C  = 105 K ferromagnet, has attracted much attention in recent years, because it develops a pronounced metamagnetic anomaly below T C for magnetic fields applied in the crystallographic ab-plane. The metamagnetic transition moves to higher fields for lower temperatures and splits into a double anomaly at critical fields H c1 = 2.3 T and H c2 = 2.8 T, respectively. Here, we report a detailed study of the different components of the magnetization vector as a function of temperature, applied magnetic field, and varying angle in Sr4Ru3O10. We discover for the first time a reduction of the magnetic moment in the plane of rotation at the metamagnetic transition. The anomaly shifts to higher fields by rotating the field from H ⊥ c to H || c. We compare our experimental findings with numerical simulations based on spin reorientation models taking into account magnetocrystalline anisotropy, Zeeman effect and antisymmetric exchange interactions. While Magnetocrystalline anisotropy combined with a Zeeman term are sufficient to explain a metamagnetic transition in Sr4Ru3O10, a Dzyaloshinskii-Moriya term is crucial to account for the reduction of the magnetic moment as observed in the experiments.

journal_name

Sci Rep

journal_title

Scientific reports

authors

Weickert F,Civale L,Maiorov B,Jaime M,Salamon MB,Carleschi E,Strydom AM,Fittipaldi R,Granata V,Vecchione A

doi

10.1038/s41598-017-03648-2

subject

Has Abstract

pub_date

2017-06-20 00:00:00

pages

3867

issue

1

issn

2045-2322

pii

10.1038/s41598-017-03648-2

journal_volume

7

pub_type

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