Abstract：
:We demonstrated modulation of charge carrier densities in all-solution-processed organic field-effect transistors (OFETs) by modifying the injection properties with self-assembled monolayers (SAMs). The all-solution-processed OFETs based on an n-type polymer with inkjet-printed Ag electrodes were fabricated as a test platform, and the injection properties were modified by the SAMs. Two types of SAMs with different dipole direction, thiophenol (TP) and pentafluorobenzene thiol (PFBT) were employed, modifying the work function of the inkjet-printed Ag (4.9 eV) to 4.66 eV and 5.24 eV with TP and PFBT treatments, respectively. The charge carrier densities were controlled by the SAM treatment in both dominant and non-dominant carrier-channel regimes. This work demonstrates that control of the charge carrier densities can be efficiently achieved by modifying the injection property with SAM treatment; thus, this approach can achieve polarity conversion of the OFETs.
journal_name
Sci Repjournal_title
Scientific reportsauthors
Roh J,Lee T,Kang CM,Kwak J,Lang P,Horowitz G,Kim H,Lee Cdoi
10.1038/srep46365subject
Has Abstractpub_date
2017-04-12 00:00:00pages
46365issn
2045-2322pii
srep46365journal_volume
7pub_type
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