Abstract:
:Inhomogeneity in the ground state is an intriguing, emergent phenomenon in magnetism. Recently, it has been observed in the magnetostructural channel of the geometrically frustrated α-NaMnO2, for the first time in the absence of active charge degrees of freedom. Here we report an in-depth numerical and local-probe experimental study of the isostructural sister compound CuMnO2 that emphasizes and provides an explanation for the crucial differences between the two systems. The experimentally verified, much more homogeneous, ground state of the stoichiometric CuMnO2 is attributed to the reduced magnetoelastic competition between the counteracting magnetic-exchange and elastic-energy contributions. The comparison of the two systems additionally highlights the role of disorder and allows the understanding of the puzzling phenomenon of phase separation in uniform antiferromagnets.
journal_name
Sci Repjournal_title
Scientific reportsauthors
Zorko A,Kokalj J,Komelj M,Adamopoulos O,Luetkens H,Arčon D,Lappas Adoi
10.1038/srep09272subject
Has Abstractpub_date
2015-03-19 00:00:00pages
9272issn
2045-2322pii
srep09272journal_volume
5pub_type
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