Manipulating size of Li3V2(PO4)3 with reduced graphene oxide: towards high-performance composite cathode for lithium ion batteries.

Abstract:

:Lithium vanadium phosphate (Li3V2(PO4)3, LVP)/reduced graphene oxide (rGO) composite is prepared with a rheological method followed by heat treatment. The size and interface of LVP particles, two important merits for a cathode material, can be effectively tuned by the rGO in the composite, which plays as surfactant to assist sol-gelation and simultaneously as conductive carbon coating. As a consequence, the composite with 7.0 ± 0.4 wt.% rGO shows a capacity of 141.6 mAh g(-1) at 0.075 C, and a rate capacity of 119.0 mAh g(-1) at 15 C with respect to the mass of LVP/rGO composite, and an excellent cycling stability that retains 98.7% of the initial discharge capacity after 50 cycles. The improved electrochemical performance is attributed to the well-controlled rGO content that yields synergic effects between LVP and rGO. Not only do the rGO sheets reduce the size of LVP particles that favor the Li(+) ion migration and the electron transfer during charging and discharging, but also contribute to the reversible lithium ions storage.

journal_name

Sci Rep

journal_title

Scientific reports

authors

Zhu X,Yan Z,Wu W,Zeng W,Du Y,Zhong Y,Zhai H,Ji H,Zhu Y

doi

10.1038/srep05768

subject

Has Abstract

pub_date

2014-08-29 00:00:00

pages

5768

issn

2045-2322

pii

srep05768

journal_volume

4

pub_type

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